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In ACS applied materials & interfaces ; h5-index 147.0

Aerosol jet printing (AJP) is a promising noncontact direct ink writing technology that enables flexible and conformal electronic devices to be fabricated onto planar and nonplanar substrates with higher resolution and less waste. Despite possessing many advantages, the limited electrical performance of microelectronic devices caused by the poor printing quality is still the greatest hurdle to overcome for AJP technology. With the motivation to improve the printing quality, a novel hybrid machine learning method is proposed to analyze and optimize the AJP process based on the deposited droplet morphology in this study. The proposed method consists of classic machine learning approaches, including space-filling-based experimental design, clustering, classification, regression, and multiobjective optimization. In the proposed method, a two-dimensional (2D) design space is fully explored using a Latin hypercube sampling approach for experimental design, and a K-means clustering approach is employed to reveal the cause-effect relationship between the deposited droplet morphology and printed line characteristics. Following that, an optimal operating window with respect to the deposited droplet morphology is identified using a support vector machine to ensure the printing quality in a design space. Finally, to achieve high-controllability and sufficient-thickness droplets, Gaussian process regression is adopted to develop the process model of droplet geometrical properties, and the deposited droplet morphology is optimized under dual conflicting objectives of customizing the droplet diameter and maximizing droplet thickness. Different from previous printing quality optimization approaches, the proposed method enables a systemic investigation on the formation mechanisms of printed line characteristics, and the printing quality is fundamentally optimized based on the deposited droplet morphology. Moreover, data-driven-based characteristics can help the proposed approach serve as a guideline for printing quality optimization in other noncontact direct ink writing technologies.

Zhang Haining, Hong Enhang, Chen Xindong, Liu Zhixin

2023-Mar-09

aerosol jet printing, droplet morphology, machine learning, noncontact direct ink writing, printing quality optimization